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Optimizing Cathode Structure for Enhanced Electrochemical Performance Using 3D-printed Lattice Structures
- Program: Materials Science and Engineering
- Course: EN.510.434 MSE Senior Design
- Year: 2025
Project Description:
This project aims to improve the performance of solid-state batteries by redesigning the cathode structure using 3D printing. Traditional cathodes limit ion and electron transport due to disorganized internal pathways. To address this, we use 3D-printed polymer lattice molds made from polycarbonate-carbon fiber (PC-CF) to guide the structure of lithium iron phosphate (LFP) cathodes. The PC-CF decomposes during sintering, leaving behind organized channels that enhance conductivity. We optimized printing parameters using the Prusa i3 Mk3S+ and tested materials using optical microscopy, DSC/TGA, and Raman spectroscopy. This method allows precise control over porosity and tortuosity to improve battery efficiency, durability, and safety.